The top-of-atmosphere net radiative effect of convective anvils is estimated to be close to zero and arises from a balance of significant short-wave cooling and long-wave warming over a complex diurnal cycle. When anvils are optically thick, the cooling due to daytime scattering of shortwave solar radiation dominates. In contrast, optically thin anvils have weaker scattering of solar radiation, so longwave warming becomes the dominant effect. Hence, it is essential to understand the controls of anvil radiative properties over the convective lifecycle, which arises from a complex interplay of convective cloud dynamics and microphysics. The convective mass flux modulates anvil extent, and changes in ice crystal size and morphology affect anvil lifetime and radiative properties. Convective anvils have been proposed to respond to global warming (cloud feedbacks) and anthropogenic aerosols (aerosol-cloud interactions). However, the associated uncertainties remain large and key relevant processes are not represented in the current generation of climate models. Emerging kilometre-scale climate models present new opportunities to examine these effects at the process level.In this work we bring together multiple research strands to quantify the controls of convective anvil clouds and associated radiative effects over the convective lifecycle towards understanding its sensitivity to climate and air pollution changes. We use the tobac cloud tracking framework to track convective cores and associated anvils in 4D across regional and global km-scale ICON model simulations which allows us to quantify the link between convective mass flux, anvil extent and anvil radiative properties. We apply this framework to regional high-resolution simulation of ICON coupled to HAM-lite, our reduced complexity aerosol model derived from the microphysical aerosol scheme HAM [Weiss et al., GMD, 2025], to explore the sensitivity of anvils and their radiative effects to aerosol perturbations in the context of the ORCHESTRA/EarthCARE Model Intercomparison Project (ECOMIP) as well as the TRACER campaign MIP. We find that an increase in aerosol increases cloud droplet numbers, suppresses warm rain formation, increases convective mass flux and thereby upper tropospheric ice water content and will discuss how these changes translate into anvil cloud radiative effects. Prototype next generation km-scale climate models are implicitly already including such anvil radiative effects; however, these currently remain unconstrained by observations. We develop novel observational constraints on the convective anvil cloud lifecycle through consistent tracking of convection using the tobac-flow cloud tracking framework [Jones et al., 2024] between MSG SEVIRI observations and forward simulated geostationary satellite radiances from ICON model output. This reveals that deep convective systems in ICON grow too fast and show a faster dissipation of thick to thin anvils than observations, which affects their radiative effects. Our work provides novel approaches to improve our understanding of aerosol effects on convective clouds and climate.